Abstract
It is explicitly shown, for optical processes arbitrarily comprising two-, three- or four-photon interactions, that the sum over all matter states of any optical susceptibility is exactly zero. The result remains true even in frequency regions where damping is prominent. Using a quantum electrodynamical framework to render the photonic nature of the fundamental interactions, the result emerges in the form of a traceless operator in Hilbert space. The generality of the sum rule and its significance as a thermodynamic limit are discussed, and the applicability to real systems is assessed.
| Original language | English |
|---|---|
| Pages (from-to) | 59-62 |
| Number of pages | 4 |
| Journal | Journal of Optics B: Quantum and Semiclassical Optics |
| Volume | 6 |
| Issue number | 1 |
| DOIs | |
| Publication status | Published - 3 Nov 2003 |