The theory of double-beam three-photon absorption. II. Polarization ratio analysis

David L. Andrews

doi:10.1063/1.444958

The theory of double-beam three-photon absorption. II. Polarization ratio analysis

David L. Andrews

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Abstract

This paper further develops the theory of double‐beam three‐photon spectroscopy introduced in part I. A much simpler method than that described previously is proposed for the experimental characterization of the three‐photon excited states, where measurement of two polarization ratios alone suffices for a complete analysis. A comprehensive classification of the excited state symmetries is provided for the common molecular point groups.

Original language	English
Pages (from-to)	1731-1734
Journal	The Journal of Chemical Physics
Volume	78
Issue number	4
DOIs	https://doi.org/10.1063/1.444958
Publication status	Published - 1 Jan 1983

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title = "The theory of double-beam three-photon absorption. II. Polarization ratio analysis",

abstract = "This paper further develops the theory of double‐beam three‐photon spectroscopy introduced in part I. A much simpler method than that described previously is proposed for the experimental characterization of the three‐photon excited states, where measurement of two polarization ratios alone suffices for a complete analysis. A comprehensive classification of the excited state symmetries is provided for the common molecular point groups.",

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AB - This paper further develops the theory of double‐beam three‐photon spectroscopy introduced in part I. A much simpler method than that described previously is proposed for the experimental characterization of the three‐photon excited states, where measurement of two polarization ratios alone suffices for a complete analysis. A comprehensive classification of the excited state symmetries is provided for the common molecular point groups.

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